NV-centers in diamond optical magnetometry utilizes completely new “quantum sensing” where we interrogate quantum states of the NV center and use it for sensing of extremely weak magnetic fields. This development will allow us to interrogate fragile states in quantum materials, such as topological insulators, unconventional superconductors and various artificial hybrid structures. Here we are specifically interested in materials and technologies relevan for Quantum Information Science (QIS), which is emerging as the next Big Effort among various agencies, DOE including.